Quantification of cooking organic aerosol in the indoor environment using aerodyne aerosol mass spectrometers

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dc.contributor.author Katz, Erin F.
dc.contributor.author Guo, Hongyu
dc.contributor.author Campuzano-Jost, Pedro
dc.contributor.author Day, Douglas A.
dc.contributor.author Brown, Wyatt L.
dc.contributor.author Boedicker, Erin
dc.contributor.author Pothier, Matson
dc.contributor.author Lunderberg, David M.
dc.contributor.author Patel, Sameer
dc.contributor.author Patel, Kanan
dc.contributor.author Hayes, Patrick L.
dc.contributor.author Avery, Anita
dc.contributor.author Hildebrandt Ruiz, Lea
dc.contributor.author Goldstein, Allen H.
dc.contributor.author Vance, Marina E.
dc.contributor.author Farmer, Delphine K.
dc.contributor.author Jimenez, Jose L.
dc.contributor.author DeCarlo, Peter F.
dc.coverage.spatial United Kingdom
dc.date.accessioned 2012-09-26T07:22:33Z
dc.date.available 2012-09-26T07:22:33Z
dc.date.issued 2021-06
dc.identifier.citation Katz, Erin F.; Guo, Hongyu; Campuzano-Jost, Pedro; Day, Douglas A.; Brown, Wyatt L.; Boedicker, Erin; Pothier, Matson; Lunderberg, David M.; Patel, Sameer; Patel, Kanan; Hayes, Patrick L.; Avery, Anita; Hildebrandt Ruiz, Lea; Goldstein, Allen H.; Vance, Marina E.; Farmer, Delphine K.; Jimenez, Jose L. and DeCarlo, Peter F., "Quantification of cooking organic aerosol in the indoor environment using aerodyne aerosol mass spectrometers", Aerosol Science and Technology, DOI: 10.1080/02786826.2021.1931013, Jun. 2021. en_US
dc.identifier.issn 0278-6826
dc.identifier.issn 1521-7388
dc.identifier.uri https://doi.org/10.1080/02786826.2021.1931013
dc.identifier.uri https://repository.iitgn.ac.in/handle/123456789/6683
dc.description.abstract The Aerodyne aerosol mass spectrometer (AMS) is used extensively to study the composition of non-refractory submicron aerosol composition during atmospheric field studies. During two recent studies of indoor environments, HOMEChem and ATHLETIC, the default ambient organic aerosol AMS quantification parameters resulted in a large discrepancy with co-located instruments while sampling cooking organic aerosol (COA). Instruments agreed within uncertainty estimates during all other sampling periods. Assuming a collection efficiency (CE) of unity, adjustments to the AMS relative ionization efficiency (RIE) were required to reach agreement with co-located instruments. The range of RIECOA observed (ATHLETIC: RIECOA 4.26-4.96, HOMEChem: RIECOA 4.70-6.50) was consistent with RIE measured in the laboratory for cooking-specific molecules. These results agree with prior AMS studies which have indicated that more oxidized outdoor ambient organic aerosol has a relatively constant RIE of 1.4 0.3 while more reduced organics have higher RIE. The applicability of a higher RIE was considered for two ambient datasets, and agreement between the AMS and colocated instruments improved when an increased response factor (RIE CE) was applied to positive matrix factorization-derived primary organic aerosol (POA). Based on the observations presented here and the literature, we recommend AMS users consider applying RIECOA 4.2 to source and indoor studies of COA and evaluate a higher POA response factor of the order of 1.5 in outdoor studies at urban background sites, and 2 at sites impacted by fresh sources. This study aims to improve AMS quantification methodology
dc.description.statementofresponsibility by Erin F. Katz, Hongyu Guo, Pedro Campuzano-Jost, Douglas A. Day, Wyatt L. Brown, Erin Boedicker, Matson Pothier, David M. Lunderberg, Sameer Patel, Kanan Patel, Patrick L. Hayes, Anita Avery, Lea Hildebrandt Ruiz, Allen H. Goldstein, Marina E. Vance, Delphine K. Farmer, Jose L. Jimenez, and Peter F. DeCarlo.
dc.language.iso en_US en_US
dc.publisher Taylor and Francis en_US
dc.title Quantification of cooking organic aerosol in the indoor environment using aerodyne aerosol mass spectrometers en_US
dc.type Article en_US
dc.relation.journal Aerosol Science and Technology


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