Plasmon-based small-molecule activation: a new dawn in the field of solar-driven chemical transformation

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dc.contributor.author Joshi, Gayatri
dc.contributor.author Mir, Ab Qayoom
dc.contributor.author Layek, Arkaprava
dc.contributor.author Ali, Afsar
dc.contributor.author Aziz, Sk. Tarik
dc.contributor.author Khatua, Saumyakanti
dc.contributor.author Dutta, Arnab
dc.coverage.spatial United States of America
dc.date.accessioned 2022-01-28T07:49:27Z
dc.date.available 2022-01-28T07:49:27Z
dc.date.issued 2022-01
dc.identifier.citation Joshi, Gayatri; Mir, Ab Qayoom; Layek, Arkaprava; Ali, Afsar; Aziz, Sk. Tarik; Khatua, Saumyakanti and Dutta, Arnab, “Plasmon-based small-molecule activation: a new dawn in the field of solar-driven chemical transformation”, ACS Catalysis, DOI: 10.1021/acscatal.1c05245, vol. 12, no. 2, pp. 1052-1067, Jan. 2022. en_US
dc.identifier.issn 2155-5435
dc.identifier.uri https://doi.org/10.1021/acscatal.1c05245
dc.identifier.uri https://repository.iitgn.ac.in/handle/123456789/7423
dc.description.abstract Gold- and silver-based plasmonic materials have emerged as game changers in the field of solar-driven small-molecule activation because of their enhanced and broadly tunable absorption cross sections. This review essays the cutting-edge research in the field of plasmon-mediated small-molecule activation while highlighting the role of plasmonic nanostructures as photosensitizers, leading to the advent of numerous photocatalytic materials. Here we initiate the discussion with a basic overview of plasmonic optical properties, followed by a detailed analysis of three major categories of plasmon-catalyst hybrid constructs, namely, single-metal plasmonic materials, plasmon-semiconductor/metal-derived systems, and the recently developed plasmon-molecular catalyst assemblies. We also narrate the challenges faced in this nascent research field while depicting the scope of future development by implementing rational modifications of the plasmonic material and/or the cocatalyst to develop innovative hybrid constructs with divergent functionalities.
dc.description.statementofresponsibility by Gayatri Joshi, Ab Qayoom Mir, Arkaprava Layek, Afsar Ali, Sk. Tarik Aziz, Saumyakanti Khatua and Arnab Dutta
dc.format.extent vol. 12, no. 2, pp. 1052-1067
dc.language.iso en_US en_US
dc.publisher American Chemical Society en_US
dc.subject Plasmon en_US
dc.subject Small-molecule activation en_US
dc.subject Single-metal plasmon en_US
dc.subject Plasmon?semiconductor assembly en_US
dc.title Plasmon-based small-molecule activation: a new dawn in the field of solar-driven chemical transformation en_US
dc.type Article en_US
dc.relation.journal ACS Catalysis


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