Apurv Chaitanya, N.N.Apurv ChaitanyaAadhi, A.A.AadhiSingh, R. P.R. P.SinghSamanta, G. K.G. K.Samanta2025-08-302025-08-302014-09-1510.1364/OL.39.0054192-s2.0-84907168771http://repository.iitgn.ac.in/handle/IITG2025/21238We report on experimental realization of optimum focusing condition for type-I second-harmonic generation (SHG) of high-power, ultrafast laser in "thick" nonlinear crystal. Using single-pass, frequency doubling of a 5 W Yb-fiber laser of pulse width ~260 fs at repetition rate of 78 MHz in a 5-mm-long bismuth triborate (BIBO) crystal we observed that the optimum focusing condition is more dependent on the birefringence of the crystal than its group-velocity mismatch (GVM). A theoretical fit to our experimental results reveals that even in the presence of GVM, the optimum focusing condition matches the theoretical model of Boyd and Kleinman, predicted for continuous-wave and long-pulse SHG. Using a focusing factor of ξ = 1.16 close to the estimated optimum value of ξ = 1.72 for our experimental conditions, we generated 2.25 W of green radiation of pulse width 176 fs with single-pass conversion efficiency as high as 46.5%. Our study also verifies the effect of pulse narrowing and broadening of angular phasematching bandwidth of SHG at tighter focusing. This study signifies the advantage of SHG in "thick" crystal in controlling SH-pulse width by changing the focusing lens while accessing high conversion efficiency and broad angular phase-matching bandwidth.falseArticle153947945419-542215 September 201439arJournal36